Mid-Infrared Intersubband Cavity Polaritons in Flexible Single Quantum Well

Nano Lett. 2023 Apr 12;23(7):2890-2897. doi: 10.1021/acs.nanolett.3c00251. Epub 2023 Mar 31.

Abstract

Strong and ultrastrong coupling between intersubband transitions in quantum wells and cavity photons have been realized in mid-infrared and terahertz spectral regions. However, most previous works employed a large number of quantum wells on rigid substrates to achieve coupling strengths reaching the strong or ultrastrong coupling regime. In this work, we experimentally demonstrate ultrastrong coupling between the intersubband transition in a single quantum well and the resonant mode of photonic nanocavity at room temperature. We also observe strong coupling between the nanocavity resonance and the second-order intersubband transition in a single quantum well. Furthermore, we implement for the first time such intersubband cavity polariton systems on soft and flexible substrates and demonstrate that bending of the single quantum well does not significantly affect the characteristics of the cavity polaritons. This work paves the way to broaden the range of potential applications of intersubband cavity polaritons including soft and wearable photonics.

Keywords: flexible substrate; intersubband transition; light−matter interaction; mid-infrared; polariton; semiconductor quantum well; ultrastrong coupling.