Liquid scintillation efficiencies, gamma-ray emission intensities, and half-life for Gd-153

Appl Radiat Isot. 2024 Jan:203:111108. doi: 10.1016/j.apradiso.2023.111108. Epub 2023 Nov 9.

Abstract

Gadolinium-153 was standardized for activity by live-timed anticoincidence counting and an ampoule was submitted to the international reference system (SIR). Absolute emission intensities for the main γ rays were determined with calibrated high-purity germanium (HPGe) and lithium-drifted silicon (Si(Li)) detectors. A revised decay scheme is indicated, with no probability of direct electron capture to the 153Eu ground state. Triple-to-double coincidence ratio (TDCR) efficiency curves indicate that the revised decay scheme is consistent with experiment. Half-life measurements agree with a previous NIST determination and show no sensitivity to chemical environment.

Keywords: Activity standard; Decay scheme; Efficiency tracing; Electron capture; Intercomparison; International reference system; Nuclear decay data; TDCR.