Identifying the electronic character and role of the Mn states in the valence band of (Ga,Mn)As

Phys Rev Lett. 2013 Aug 30;111(9):097201. doi: 10.1103/PhysRevLett.111.097201. Epub 2013 Aug 27.

Abstract

We report high-resolution hard x-ray photoemission spectroscopy results on (Ga,Mn)As films as a function of Mn doping. Supported by theoretical calculations we identify, for both low (1%) and high (13%) Mn doping values, the electronic character of the states near the top of the valence band. Magnetization and temperature-dependent core-level photoemission spectra reveal how the delocalized character of the Mn states enables the bulk ferromagnetic properties of (Ga,Mn)As.