In situ Electrical Impedance Tomography for Visualizing Water Transportation in Hygroscopic Aerogels

Adv Sci (Weinh). 2024 May 14:e2402676. doi: 10.1002/advs.202402676. Online ahead of print.

Abstract

The global water crisis demands immediate attention, and atmospheric water harvesting (AWH) provides a viable alternative. However, studying the real-time subtle relationship between water absorption, diffusion, and internal structure for hygroscopic materials is challenging. Herein, a dynamic visualization technique is proposed that utilizes an in situ electrical impedance tomography (EIT) system and a precise reconstruction algorithm to achieve real-time monitoring of the water sorption process within aerogels from an internal microstructural perspective. These results can be inferred that composites' pore sizes affecting the kinetics of their moisture absorption. In addition, the diffusion path of moisture absorption and the distribution of stored moisture inside aerogels exhibit intrinsic self-selective behavior, where the fiber skeleton of the aerogel plays a crucial role. In summary, this work proposes a generic EIT-based technique for the in situ and dynamic monitoring of the hygroscopic process, pointing to an entirely new approach regarding research on AWH materials.

Keywords: cellulose nanocrystals; electrical impedance tomography; emulsion template; moisture absorption; water diffusion.